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Applied Physics Letters : An in situ electrical study on primary hydrogen spillover from nanocatalysts to amorphous carbon support

By Chikai Lin, Zhenzhen Yang, Tao Xu, and Yufeng Zhao

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Book Id: WPLBN0002169238
Format Type: PDF eBook :
File Size: Serial Publication
Reproduction Date: 10 December 2008

Title: Applied Physics Letters : An in situ electrical study on primary hydrogen spillover from nanocatalysts to amorphous carbon support  
Author: Chikai Lin, Zhenzhen Yang, Tao Xu, and Yufeng Zhao
Volume: Issue : December 2008
Language: English
Subject: Science, Physics, Natural Science
Collections: Periodicals: Journal and Magazine Collection (Contemporary), Applied Physics Letters Collection
Historic
Publication Date:
Publisher: American Institute of Physics

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Zhenzhen Yang, Tao Xu, And Yufeng Zha, C. L. (n.d.). Applied Physics Letters : An in situ electrical study on primary hydrogen spillover from nanocatalysts to amorphous carbon support. Retrieved from http://hawaiilibrary.net/


Description
Description: Primary hydrogen spillover has been studied using a unique electrical method. We observed that at ambient temperature, when a discontinuous nanogranular Pd film is on the top of an amorphous carbon film, the electrical conductance of the carbon film decreases in pressurized hydrogen. In comparison, in the absence of this Pd layer, the conductance of the carbon film remains unchanged in pressurized hydrogen. The observed decrease in the current in the Pd/carbon structure is ascribed to the hydrogenation of the dangling carbon bonds and sp2-sp3 transition in the amorphous carbon by the primary spillover hydrogen atoms from Pd nanoclusters.

 

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